Onset of Bloch oscillations in the almost-strong-field regime

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Reislöhner, J.; Kim, D.; Babushkin, I.; Pfeiffer, A.N.: Onset of Bloch oscillations in the almost-strong-field regime. In: Nature Communications 13 (2022), Nr. 1, 7716. DOI: https://doi.org/10.1038/s41467-022-35401-3

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Abstract: 
In the field of high-order harmonic generation from solids, the electron motion typically exceeds the edge of the first Brillouin zone. In conventional nonlinear optics, on the other hand, the excursion of band electrons is negligible. Here, we investigate the transition from conventional nonlinear optics to the regime where the crystal electrons begin to explore the first Brillouin zone. It is found that the nonlinear optical response changes abruptly already before intraband currents due to ionization become dominant. This is observed by an interference structure in the third-order harmonic generation of few-cycle pulses in a non-collinear geometry. Although approaching Keldysh parameter γ = 1, this is not a strong-field effect in the original sense, because the iterative series still converges and reproduces the interference structure. The change of the nonlinear interband response is attributed to Bloch motion of the reversible (or transient or virtual) population, similar to the Bloch motion of the irreversible (or real) population which affects the intraband currents that have been observed in high-order harmonic generation.
License of this version: CC BY 4.0 Unported
Document Type: Article
Publishing status: publishedVersion
Issue Date: 2022
Appears in Collections:Fakultät für Mathematik und Physik

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1 image of flag of United States United States 9 37.50%
2 image of flag of Germany Germany 9 37.50%
3 image of flag of Russian Federation Russian Federation 3 12.50%
4 image of flag of Indonesia Indonesia 2 8.33%
5 image of flag of China China 1 4.17%

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