Cavity enhanced detection of cold molecules

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Schnars, Jannis: Cavity enhanced detection of cold molecules. Hannover : Gottfried Wilhelm Leibniz Universität, Diss., 2022, xi, 127 S., DOI: https://doi.org/10.15488/12371

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Sum total of downloads: 385




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Abstract: 
Cold quantum gases are versatile tools not only to investigate quantum many-body physics and ultracold chemistry, but also for testing fundamental theories. Many degenerate quantum gases, however, consist of atoms and provide only short-range interactions between different particles limiting research opportunities. Hence, shortly after the production of the first atomic gases an interest arose in ensembles of cold polar molecules that exhibit adjustable long-range anisotropic dipole-dipole interactions to expand research fields further. Loading such a molecular cloud into an optical lattice provides an excellent experimental control regarding particle-particle interactions and to simulate condensed matter physics.Experiments with cold quantum gases require imaging techniques to determine properties like the number of atoms and molecules or the position of single particles. For atomic ensembles, absorption or fluorescence techniques are often utilised since atoms usually provide closed cycling transitions allowing to scatter a large number of photons for the imaging signal. The internal level structure of molecules, though, is more complex compared to atoms due to additional rovibrational states and many molecules do not provide closed cycling transitions. For these molecules new imaging techniques need to be developed.In the first part of the thesis a theoretical background of the imaging technique is provided, starting with a classical approach. The advantages of a classical theory are an intuitive understanding of the detection method and an applicability to spherical nanoparticles, which can then be utilised as test objects for the proposed imaging scheme. The resolution capability of the detection technique is discussed and the important role of small cavity waists for high resolutions is highlighted. In a next step, a full quantum mechanical approach is presented and compared to the classical theory. It is shown that both theories are equivalent except for vacuum fluctuations, a pure quantum physical effect important to determine quantum noise correctly.After introducing theoretical backgrounds, cavity geometries suitable for the detection of molecules are discussed. Properties, directly important for the imaging process, e.\;g. waist, mode number and linewidth, and technical aspects like misalignment sensitivity are taken into account. A simultaneous optimisation of all these properties is not possible since they are partially contradicting each other. However, a balance between these different aspects is found. Two cavity geometrics, feasible for imaging NaK molecules, a hemispherical resonator and a concentric cavity are proposed.Finally, an experimental setup to demonstrate the general feasibility of the imaging technique is developed. Titania and silver are identified as materials for nanoparticles best suited to imitate NaK molecules. Imaging resonators are designed and an alignment procedure for these cavities is presented.
License of this version: CC BY 3.0 DE
Document Type: DoctoralThesis
Publishing status: publishedVersion
Issue Date: 2022
Appears in Collections:Fakultät für Mathematik und Physik
Dissertationen

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1 image of flag of Germany Germany 115 29.87%
2 image of flag of United States United States 99 25.71%
3 image of flag of China China 23 5.97%
4 image of flag of Czech Republic Czech Republic 22 5.71%
5 image of flag of Russian Federation Russian Federation 17 4.42%
6 image of flag of India India 13 3.38%
7 image of flag of Switzerland Switzerland 12 3.12%
8 image of flag of Italy Italy 11 2.86%
9 image of flag of United Kingdom United Kingdom 11 2.86%
10 image of flag of Singapore Singapore 9 2.34%
    other countries 53 13.77%

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