Creep in reactive colloidal gels: A nanomechanical study of cement hydrates

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Haist, M.; Divoux, T.; Krakowiak, K.J.; Skibsted, J.; Pellenq, R.J.-M. et al.: Creep in reactive colloidal gels: A nanomechanical study of cement hydrates. In: Physical review research 3 (2021), 043127. DOI: https://doi.org/10.1103/PhysRevResearch.3.043127

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Sum total of downloads: 87




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Abstract: 
From soft polymeric gels to hardened cement paste, amorphous solids under constant load exhibit a pronounced time-dependent deformation called creep. The microscopic mechanism of such a phenomenon is poorly understood in amorphous materials and constitutes an even greater challenge in densely packed and chemically reactive granular systems. Both features are prominently present in hydrating cement pastes composed of calcium silicate hydrate (C-S-H) nanoparticles, whose packing density increases as a function of time, while cement hydration is taking place. Performing nanoindentation tests and porosity measurements on a large collection of samples at various stages of hydration, we show that the creep response of hydrating cement paste is mainly controlled by the interparticle distance and results from slippage between (C-S-H) nanoparticles. Our findings provide a unique insight into the microscopic mechanism underpinning the creep response in aging granular materials, thus paving the way for the design of concrete with improved creep resistance.
License of this version: CC BY 4.0 Unported
Document Type: Article
Publishing status: publishedVersion
Issue Date: 2021
Appears in Collections:Fakultät für Bauingenieurwesen und Geodäsie

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pos. country downloads
total perc.
1 image of flag of Germany Germany 30 34.48%
2 image of flag of United States United States 18 20.69%
3 image of flag of China China 18 20.69%
4 image of flag of Latvia Latvia 5 5.75%
5 image of flag of No geo information available No geo information available 3 3.45%
6 image of flag of Sweden Sweden 3 3.45%
7 image of flag of India India 2 2.30%
8 image of flag of Austria Austria 2 2.30%
9 image of flag of South Africa South Africa 1 1.15%
10 image of flag of Belgium Belgium 1 1.15%
    other countries 4 4.60%

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